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Journal Articles Chemical Reviews Year : 2021

Aqueous Corrosion of Glasses, Crystalline Ceramics, and Metals

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1
Gerald Frankel
  • Function : Author
John Vienna
  • Function : Author
Jie Lian
  • Function : Author
Xiaolei Guo
  • Function : Author
Seong Kim
  • Function : Author
J. Du
  • Function : Author
Joseph Ryan
Jianwei Wang
  • Function : Author
Wolfgang Windl
  • Function : Author
Christopher Taylor
John Scully
  • Function : Author

Abstract

High-level radioactive waste is accumulating at temporary storage locations around the world and will eventually be placed in deep geological repositories. The waste forms and containers will be constructed from glass, crystalline ceramic, and metallic materials, which will eventually come into contact with water, considering that the period of performance required to allow sufficient decay of dangerous radionuclides is on the order of 10E5-10E6 years. Corrosion of the containers and waste forms in the aqueous repository environment is therefore a concern. This Review describes the recent advances of the field of materials corrosion that are relevant to fundamental materials science issues associated with the long-term performance assessment and the design of materials with improved performance, where performance is defined as resistance to aqueous corrosion. Glass, crystalline ceramics, and metals are discussed separately, and the near-field interactions of these different material classes are also briefly addressed. Finally, recommendations for future directions of study are provided.
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Dates and versions

cea-03577575 , version 1 (16-02-2022)

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Gerald Frankel, John Vienna, Jie Lian, Stephane Gin, Xiaolei Guo, et al.. Aqueous Corrosion of Glasses, Crystalline Ceramics, and Metals. Chemical Reviews, 2021, 121, pp.12327-12383. ⟨10.1021/acs.chemrev.0c00990⟩. ⟨cea-03577575⟩
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