Ultrafast Structural Dynamics of Nanoparticles in Intense Laser Fields
Toshiyuki Nishiyama
(1)
,
Yoshiaki Kumagai
(2)
,
Akinobu Niozu
(1, 3)
,
Hironobu Fukuzawa
(2, 4)
,
Koji Motomura
(2)
,
Maximilian Bucher
(5)
,
Yuta Ito
(2)
,
Tsukasa Takanashi
(2)
,
Kazuki Asa
(1)
,
Yuhiro Sato
(1)
,
Daehyun You
(2)
,
Yiwen Li
(2)
,
Taishi Ono
(2)
,
Edwin Kukk
(6)
,
Catalin Miron
(7, 8)
,
Liviu P. Neagu
(8)
,
Carlo Callegari
(9)
,
Michele Di Fraia
(9)
,
Giorgio Rossi
(10)
,
Davide Galli
(10)
,
Tommaso Pincelli
(10)
,
Alessandro Colombo
(10)
,
Takashi Kameshima
(11)
,
Yasumasa Joti
(11)
,
Takaki Hatsui
(3)
,
Shigeki Owada
(3)
,
Tetsuo Katayama
(11)
,
Tadashi Togashi
(11)
,
Kensuke Tono
(3)
,
Makina Yabashi
(3)
,
Kazuhiro Matsuda
,
Christoph Bostedt
(5)
,
Kiyonobu Nagaya
(3)
,
Kiyoshi Ueda
(3, 2)
1
Kyoto University
2 Tohoku University [Sendai]
3 RIKEN - RIKEN - Institute of Physical and Chemical Research [Japon]
4 RIKEN - Environmental Molecular Biology Laboratory
5 ANL - Argonne National Laboratory [Lemont]
6 University of Turku
7 LIDyl - Laboratoire Interactions, Dynamiques et Lasers (ex SPAM)
8 Extreme Light Infrastructure
9 Elettra Sincrotrone Trieste
10 Dipartimento di Fisica (Milano)
11 JASRI - Japan Synchrotron Radiation Research Institute [Hyogo]
2 Tohoku University [Sendai]
3 RIKEN - RIKEN - Institute of Physical and Chemical Research [Japon]
4 RIKEN - Environmental Molecular Biology Laboratory
5 ANL - Argonne National Laboratory [Lemont]
6 University of Turku
7 LIDyl - Laboratoire Interactions, Dynamiques et Lasers (ex SPAM)
8 Extreme Light Infrastructure
9 Elettra Sincrotrone Trieste
10 Dipartimento di Fisica (Milano)
11 JASRI - Japan Synchrotron Radiation Research Institute [Hyogo]
Akinobu Niozu
- Function : Author
- PersonId : 797174
- ORCID : 0000-0002-7292-5630
Hironobu Fukuzawa
- Function : Author
- PersonId : 792708
- ORCID : 0000-0002-8283-381X
Maximilian Bucher
- Function : Author
- PersonId : 797175
- ORCID : 0000-0001-7896-473X
Catalin Miron
- Function : Author
- PersonId : 1222468
- IdHAL : catalinmiron
- ORCID : 0000-0002-8302-7158
- IdRef : 193121875
Giorgio Rossi
- Function : Author
- PersonId : 792786
- ORCID : 0000-0002-9330-7436
Alessandro Colombo
- Function : Author
- PersonId : 763771
- ORCID : 0000-0002-7950-293X
Shigeki Owada
- Function : Author
- PersonId : 780427
- ORCID : 0000-0002-1451-7612
Kensuke Tono
- Function : Author
- PersonId : 780426
- ORCID : 0000-0003-1218-3759
Makina Yabashi
- Function : Author
- PersonId : 763945
- ORCID : 0000-0002-2472-1684
Kazuhiro Matsuda
- Function : Author
- PersonId : 797176
- ORCID : 0000-0002-6576-7056
Kiyoshi Ueda
- Function : Author
- PersonId : 775654
- ORCID : 0000-0001-8051-8966
Abstract
Femtosecond laser pulses have opened new frontiers for the study of ultrafast phase transitions and
nonequilibrium states of matter. In this Letter, we report on structural dynamics in atomic clusters pumped
with intense near-infrared (NIR) pulses into a nanoplasma state. Employing wide-angle scattering with
intense femtosecond x-ray pulses from a free-electron laser source, we find that highly excited xenon
nanoparticles retain their crystalline bulk structure and density in the inner core long after the driving NIR
pulse. The observed emergence of structural disorder in the nanoplasma is consistent with a propagation
from the surface to the inner core of the clusters.