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Journal articles
Self-optimization of plasmonic nanoantennas in strong femtosecond fields
Liping Shi
1, 2
Bianca Iwan
2, 3, 4
Rana Nicolas
3, 4
Quentin Ripault
3, 4
Jose R. C. Andrade
1
Seunghwoi Han
5
Hyunwoong Kim
5
Willem Boutu
3, 4
Dominik Franz
3, 4
Torsten Heidenblut
6
Carsten Reinhardt
7
Bert Bastiaens
8
Tamas Nagy
1
Ihar Babushkin
1
Uwe Morgner
1
Seung-Woo Kim
9
Günter Steinmeyer
10
Hamed Merdji
3, 4
Milutin Kovacev
1
4
ATTO - Attophysique
IRAMIS - Institut Rayonnement Matière de Saclay, LIDyl - Laboratoire Interactions, Dynamiques et Lasers (ex SPAM)
Liping Shi 1, 2
Author
Bianca Iwan 2, 3, 4
Author
Rana Nicolas 3, 4
Author
Quentin Ripault 3, 4
Author
Dominik Franz 3, 4
Author
Torsten Heidenblut 6
Author
Carsten Reinhardt 7
Author
Bert Bastiaens 8
Author
1
IQ - Institut für Quantenoptik [Hannover] (Welfengarten 1, Leibniz Universität, D-30167 Hannover - Germany)
- LUH - Leibniz Universität Hannover [Hannover] (Gottfried Wilhelm Leibniz Universität Hannover Welfengarten 1 D-30167 Hannover - Germany)
2
QUEST - Centre for Quantum Engineering and Space-time Research (Appelstrasse 2, 30167, Hannover, Germany - Germany)
- LUH - Leibniz Universität Hannover [Hannover] (Gottfried Wilhelm Leibniz Universität Hannover Welfengarten 1 D-30167 Hannover - Germany)
3
LIDyl - Laboratoire Interactions, Dynamiques et Lasers (ex SPAM) (LIDYL, CEA, CNRS, Université Paris-Saclay, CEA Saclay 91190 Gif sur Yvette - France)
- CEA - Commissariat à l'énergie atomique et aux énergies alternatives : DRF/IRAMIS (Centre de Saclay Centre de Grenoble Centre de Cadarache etc - France)
- Université Paris-Saclay (Espace Technologique, Bat. Discovery - RD 128 - 2e ét., 91190 Saint-Aubin - France)
- CNRS - Centre National de la Recherche Scientifique : UMR9222 (France)
4
ATTO - Attophysique (France)
- IRAMIS - Institut Rayonnement Matière de Saclay (91191 Gif-sur-Yvette, France - France)
- CEA - Commissariat à l'énergie atomique et aux énergies alternatives : DRF/IRAMIS (Centre de Saclay Centre de Grenoble Centre de Cadarache etc - France)
- Université Paris-Saclay (Espace Technologique, Bat. Discovery - RD 128 - 2e ét., 91190 Saint-Aubin - France)
- LIDyl - Laboratoire Interactions, Dynamiques et Lasers (ex SPAM) (LIDYL, CEA, CNRS, Université Paris-Saclay, CEA Saclay 91190 Gif sur Yvette - France)
- CEA - Commissariat à l'énergie atomique et aux énergies alternatives : DRF/IRAMIS (Centre de Saclay Centre de Grenoble Centre de Cadarache etc - France)
- Université Paris-Saclay (Espace Technologique, Bat. Discovery - RD 128 - 2e ét., 91190 Saint-Aubin - France)
- CNRS - Centre National de la Recherche Scientifique : UMR9222 (France)
5
KAIST - Department of Electrical Engineering [Korea Advanced Institute of Science and Technology] (335 Gwahak-ro (373-1 Guseong-dong) Yuseong-gu, Daejeon 305-701 Republic of Korea - South Korea)
- KAIST - Korea Advanced Institute of Science and Technology (291 Daehak-ro, Yuseong-gu, Daejeon 34141, Republic of Korea - South Korea)
7
Laser Zentrum Hannover (France)
8
MESA+ - Institute for Nanotechnology (Faculty of Science and Technology and MESA+ P.O. Box 217, 7500 AE Enschede, The Netherlands - Netherlands)
- University of Twente [Netherlands] (Drienerlolaan 5, 7522 NB Enschede - Netherlands)
9
KAIST - Korea Advanced Institute of Science and Technology (291 Daehak-ro, Yuseong-gu, Daejeon 34141, Republic of Korea - South Korea)
10
MBI - Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie (Max-Born-Straße 2 A, 12489 Berlin - Germany)
Abstract : Plasmonic dimer nanoantennas can significantly boost the electric field strength in the gap region, allowing for a modification of the feed gap geometry by femtosecond laser illumination. Using resonant bowtie antennas to enhance the electric field of a low-fluence femtosecond oscillator, here we experimentally demonstrate highly localized reshaping of the antennas, resulting in a self-optimization of the antenna shape. From high-resolution scanning electron micrographs and two-dimensional energy dispersive x-ray maps, we analyze the near-field enhanced subwavelength ablation at the nanotips and the resulting deposition of ablated materials in the feed gap. The dominant ablation mechanism is attributed to the nonthermal transient unbonding of atoms and electrostatic acceleration of ions. This process is driven by surface plasmon enhanced electron emission, with subsequent acceleration in the vacuum. This ablation is impeded in the presence of an ambient gas. A maximum of sixfold enhancement of the third-harmonic yield is observed during the reshaping process.
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Journal articles
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https://hal-cea.archives-ouvertes.fr/cea-01613485
Contributor : Caroline Lebe <>
Submitted on : Monday, October 9, 2017 - 4:26:46 PM
Last modification on : Thursday, July 1, 2021 - 4:44:01 PM
Contributor : Caroline Lebe <>
Submitted on : Monday, October 9, 2017 - 4:26:46 PM
Last modification on : Thursday, July 1, 2021 - 4:44:01 PM
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Identifiers
- HAL Id : cea-01613485, version 1
- DOI : 10.1364/OPTICA.4.001038
Collections
CEA | CNRS | IRAMIS-LIDYL | CEA-UPSAY | IRAMIS | GS-CHIMIE | GS-ENGINEERING | INSTITUT-SCIENCES-LUMIERE
Citation
Liping Shi, Bianca Iwan, Rana Nicolas, Quentin Ripault, Jose R. C. Andrade, et al.. Self-optimization of plasmonic nanoantennas in strong femtosecond fields. Optica, Optical Society of America - OSA Publishing, 2017, 4 (9), ⟨10.1364/OPTICA.4.001038⟩. ⟨cea-01613485⟩
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